Corrected entry: The exterior shot, from behind the Harrier, towards the building shows that all the windows are mirrored glass. Harry would only have seen his reflection on the side of the building and couldn't have known where the terrorists were, or even if he knew which floor, whether there were any hostages or other innocent people inside.
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Correction: Harry had a situation-report given to him by fellow agent Faisil, who was posing as part of the news crew inside the building. This included where all the hostages and terrorists were. Faisil was very clear on where all the hostages were. As for Harry knowing where the terrorists were, he didn't. That's why he (virtually) shot up the entire floor to make sure he got as many as possible.
XIII